A Modelling Perspective of the Summer 2013 and 2014 ChArMEx/SAFMED Chemistry Intensive Campaigns: Origin of Photo-Oxidant and Aerosol Formation over the Western Mediterranean

AIR POLLUTION MODELING AND ITS APPLICATION XXIV(2016)

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摘要
During summers 2013 and 2014, two three weeks intensive campaign took place over the western Mediterranean basin in order to investigate photo-oxidant and aerosol sources over the region. Within the frame of the MISTRALS/ChArMEx (Chemistry-Aerosol Mediterranean Experiment) program and the ANR/SAFMED (Secondary Aerosol Formation in the MEDiterranean) project, this campaign included an extensive experimental set-up based on ground-based, balloon-borne, aircraft and satellite measurements. In this paper, a modeling perspective of the campaign is given, based on simulations with the regional chemistry-transport model, CHIMERE, in a configuration shaped for the Mediterranean region. Major sources of photo-oxidants, and aerosols are addressed: long range transport from continental Europe, pollution build-up from shipping emissions, marine emissions, organic aerosol formation from biogenic and anthropogenic VOC emissions, dust emissions.
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关键词
Emission Inventory, Dust Emission, Dimethyl Sulfide, Secondary Organic Aerosol, Aerosol Formation
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