Photoredox-Catalyzed α-C(sp 3 )-H Activation of Unprotected Secondary Amines: Facile Access to 1,4-Dicarbonyl Compounds

Qian Zhang
Qian Zhang
Le-Wu Zhan
Le-Wu Zhan
Wan-Ying Tang
Wan-Ying Tang
Jing Hou
Jing Hou
Bin-Dong Li
Bin-Dong Li

Organic letters, 2020.

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Abstract:

A photoredox-catalyzed α-C(sp)-H activation approach of unprotected secondary amines is reported. Such transformations provide facile access to various 1,4-dicarbonyl compounds using readily available amines and α,β-unsaturated compounds as feedstocks under air conditions. The substrate scope of this method is broad, and a wide array of f...More

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