Defect engineering of NH2-MIL-88B(Fe) using different monodentate ligands for enhancement of photo-Fenton catalytic performance of acetamiprid degradation

Yuexin Wang,Zhen Zhong,Yaseen Muhammad,Hui He,Zhongxing Zhao, Shuangxi Nie,Zhenxia Zhao

Chemical Engineering Journal（2020）

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摘要

•Ligand defects were engineered in MIL88(Fe) via different coordinations.•Ligand defects intensified adsorption ability of MIL88(Fe) towards acetamiprid.•Ligand defects improved light absorption and charge separation for MOF photocatalysis.•Ligand vacancy strengthened Fe Lewis acidity and improved Fe2+/Fe3 + redox reaction.•Pca-MIL88(Fe) greatly enhanced ACTM mineralization rate under visible light.

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关键词

Monodentate ligand strategy,Coordination mode,Ligand vacancy,Lewis acid site,photo-Fenton catalysis,Acetamiprid degradation

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