Controlling Photocatalytic Reduction Of Co2 In Ru(Ii)/Re(I) Dyads Via Linker Oxidation State

Christopher M. Brown,Thomas Auvray,Emile E. Deluca,Maria B. Ezhova,Garry S. Hanan,Michael O. Wolf

CHEMICAL COMMUNICATIONS（2020）

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摘要

Electronic communication between the linked metal centers in Ru(ii)-Re(i) dyads is tuned using the oxidation state (S and SO2) of sulfur-bridged ligands. Higher catalytic activity is seen for the SO2-bridged dyad in the photocatalytic reduction of CO2.

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