An interlaboratory collaboration to determine consensus 231 Pa/ 235 U model ages of a uranium certified reference material for nuclear forensics

Journal of Radioanalytical and Nuclear Chemistry(2020)

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摘要
Application of the 231 Pa/ 235 U radiochronometer for nuclear forensic investigations is challenged by a lack of certified reference materials with 231 Pa/ 235 U model purification dates. The Japan Atomic Energy Agency, Los Alamos National Laboratory, and Lawrence Livermore National Laboratory completed an interlaboratory study measuring 231 Pa/ 235 U model ages of New Brunswick Laboratory CRM U100. Results from independent laboratories were combined to calculate a consensus 231 Pa/ 235 U model purification date for CRM U100 of March 26, 1959 ± 237 days. This 231 Pa/ 235 U consensus date for CRM U100 may be used by the nuclear forensic community for quality control of 231 Pa/ 235 U radiochronometry measurements of unknown materials.
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关键词
Radiochronometry,Uranium,Protactinium,Radiochemistry,Mass spectrometry
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