Cloudy sky contributions to the direct aerosol effect

Atmospheric Chemistry and Physics(2020)

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摘要
Abstract. The radiative forcing of the aerosol-radiation interaction can be decomposed into clear sky and cloudy sky portions. Two sets of multi-model simulations within AeroCom, combined with observational methods, and the time evolution of aerosol emissions over the industrial era show that the contribution from cloudy sky regions is likely weak. A mean of the simulations considered is 0.01 ± 0.1 W m−2. Multivariate data analysis of results from AeroCom Phase II shows that many factors influence the strength of the cloudy sky contribution to the forcing of the aerosol-radiation interaction. Overall, single scattering albedo of anthropogenic aerosols and the interaction of aerosols with the shortwave cloud radiative effects are found to be important factors. A more dedicated focus on the contribution from the cloud free and cloud covered sky fraction respectively to the aerosol-radiation interaction will benefit the quantification of the radiative forcing and its uncertainty range.
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