Nonmetallic Metal Toward A Pressure-Induced Bad-Metal State In Two-Dimensional Cu3liru2o6

CHEMICAL COMMUNICATIONS(2020)

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摘要
The novel two-dimensional honeycomb layered Cu3LiRu2O6 exhibits Pauli-like paramagnetic and Mott variable range hopping semiconduction behaviors, which contradict the large specific-heat Sommerfeld coefficient for metals, and indicate a possible spin-excitation induced nonmetallic metal. This nonmetallic feature can be significantly suppressed by pressure toward producing a bad-metal state, as reflected by the temperature-dependent resistivity response up to 35 GPa.
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