Electron shakeoff following the e̱ṯa̱+ decay of 19Ne+ and 35Ar+ trapped ions

PHYSICAL REVIEW A(2018)

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摘要
The electron shakeoff of 19F and 35Cl atoms resulting from the e̱ṯa̱+ decay of 19Ne+ and 35Ar+ ions has been investigated using a Paul trap coupled to a time of flight recoil-ion spectrometer. The charge-state distributions of the recoiling daughter nuclei were compared to theoretical calculations based on the sudden approximation and accounting for subsequent Auger processes. The excellent agreement obtained for 35Cl is not reproduced in 19F. The shortcoming is attributed to the inaccuracy of the independent particle model employed to calculate the primary shakeoff probabilities in systems with rather low atomic numbers. This calls for more elaborate calculations, including explicitly the electron-electron correlations.
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