Exploring the electronic structure and speciation of aqueous and colloidal Pu with high energy resolution XANES and computations.

Tonya Vitova,Ivan Pidchenko,David Fellhauer,Tim Pruessmann,Sebastian Bahl,Kathy Dardenne,Tadahiro Yokosawa,Bernd Schimmelpfennig,Marcus Altmaier,Melissa Denecke,Jörg Rothe,Horst Geckeis

CHEMICAL COMMUNICATIONS（2018）

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摘要

Pu L-3 HR-XANES and FEFF9 computations provide evidence for band-like 6d states in colloidal Pu contrasting to narrow 6d states in molecular Pu(iv). Pu L-3 HR-XANES is valuable for bond length estimation in plutonyl, whereas Pu M-5 HR-XANES is an advanced tool for analysing Pu redox states and 5f unoccupied density of states.

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