Imaging the solvation of a one-dimensional solid on the molecular scale.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION(2018)
摘要
We have observed the inversion of the solvation environment of a one-dimensional solid by low-temperature scanning tunneling microscopy. Adsorption of 3-methoxy-9-diazofluorene on Ag(111) yields highly oriented supramolecular chains, which are then exposed to water molecules. The annealing of dry and water-decorated chains results in diametrically opposed outcomes. While the former simply leads to an increase in chain length and number, the latter results in a complete loss of order and produces water clusters decorated with the organic molecule.
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关键词
scanning tunneling microscopy,single-molecule studies,solvation,surface chemistry
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