Redox-Annulations of Cyclic Amines with 2-(2-Oxoethyl)malonates.
Organic letters（2018）
摘要
Amines such as 1,2,3,4-tetrahydroisoquinoline undergo redox-neutral annulations with 2-(2-oxoethyl)malonates in the presence of catalytic amounts of benzoic acid. These reactions install a fully saturated five-membered ring and provide access to structures closely related to the natural products crispine A and harmicine.
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