Catalysis of photooxidation reactions through transformation between Cu 2+ and Cu + in TiO 2 -Cu-MOF composites.

Chunjun Chen,Tianbin Wu,Dexin Yang,Pei Zhang,Huizhen Liu,Youdi Yang,Guanying Yang,Buxing Han

CHEMICAL COMMUNICATIONS（2018）

引用 37|浏览9

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摘要

Novel porous TiO2@Cu-3(BTC)(2) composites, which were synthesized using ionic liquids (ILs) as solvents, exhibited excellent activity for photooxidation of styrene to 4-aryl tetralones and promoting the Glaser coupling reaction with O-2 under light irradiation. It was discovered that the transformation between Cu2+ and Cu+ was crucial for enhancing the photocatalytic performance.

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