Evaluation of mean transit time of aerosols from the area of origin to the Arctic with 210 Pb/ 210 Po daily monitoring data.

Weihua Zhang,Baki Sadi, Christopher Rinaldo,Jing Chen, Norman Spencer,Kurt Ungar

Journal of Environmental Radioactivity(2018)

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摘要
In this study, the activity concentrations of 210Pb and 210Po on the 22 daily air filter samples, collected at CTBT Yellowknife station from September 2015 to April 2016, were analysed. To estimate the time scale of atmospheric long-range transport aerosol bearing 210Pb in the Arctic during winter, the mean transit time of aerosol bearing 210Pb from its origin was determined based on the activity ratios of 210Po/210Pb and the parent-progeny decay/ingrowth equation. The activity ratios of 210Po/210Pb varied between 0.06 and 0.21 with a median value of 0.11. The aerosol mean transit time based the activity ratio of 210Po/210Pb suggests longer mean transit time of 210Pb aerosols in winter (12 d) than in autumn (3.7 d) and spring (2.9 d).
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关键词
210Pb/210Po,Tracer,Residence time of aerosols,Arctic
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