Layered γ-Zirconium Phosphate Intercalated with Ru(bpy) 3 -Viologen Dyads as Unusual Materials for Dye-Sensitised Solar Cells: Improving Efficiency by Double Sensitisation

Maria De Victoriarodriguez,Pedro Atienzar,Olga Juanes,Juan Carlos Rodriguezubis,Ernesto Brunet,Hermenegildo Garcia

AUSTRALIAN JOURNAL OF CHEMISTRY（2014）

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摘要

The intercalation materials prepared from the laminar salt gamma-zirconium phosphate and various dyads formed from Ru(bpy)(3) and viologens were tested as photoactive components in dye-sensitised solar cells. The efficiencies significantly increased, up to 0.2 %, when the materials were treated with the panchromatic N535 dye. A mechanism for this double sensitisation process is proposed, which should enable further improvement of these gamma-ZrP-based materials as a reasonable alternative to the usual Ti-based dye-sensitised solar cells.

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关键词

physical chemistry,crystallography,electrochemistry,macromolecules,self assembly,kinetics,reaction mechanisms,biological chemistry,structure,pharmaceutical chemistry,combinatorial chemistry,sensors,combinatorial,organic chemistry,biocatalysis,density functional theory,amino acids,catalysis,biosensors,analytical chemistry,crystal structures,enzymes,inorganic chemistry,surface chemistry,colloids,ab initio calculations,nanotechnology,medicinal chemistry,spectroscopy,photochemistry,green chemistry,mass spectrometry,quantum chemistry,interfaces,proteins,ionic liquids,supramolecular chemistry,polymer chemistry,computational chemistry,educational,peptide

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