We have collected the first physics data of an experimental search for the simplest kaonic nuclear bound state, "K- pp", by the He-3(K-, n) reaction at J-PARC. We confirmed that our spectrometer system works as designed and observed clear peak structure composed of the quasi-elastic K-"n" -> K(-)n and the charge-exchange K-"p" -> k(0)n Int reactions in the forward neutron spectrum.