Photoelectrochemical CO2 reduction using a Ru(II)–Re(I) multinuclear metal complex on a p-type semiconducting NiO electrode

Go Sahara,Ryu Abe,Masanobu Higashi,Takeshi Morikawa,Kazuhiko Maeda,Yutaro Ueda,Osamu Ishitani

CHEMICAL COMMUNICATIONS（2015）

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摘要

A photocathode for CO2 reduction was successfully developed using a hybrid electrode comprising a Ru(II)-Re(I) supramolecular photocatalyst and a NiO electrode. Selective photoexcitation of the Ru photosensitizer unit of the photocatalyst at -1.2 V vs. Ag/AgNO3 selectively afforded CO with high faradaic efficiency.

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