Chirp-controlled ground-state photodissociation of Cr(CO)6

Thomas Witte,Lars Windhorn,Jake S Yeston,Marcus Motzkus,D Proch,Karlludwig Kompa

Springer Series in Chemical Physics（2003）

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摘要

Femtosecond laser excitation of the T-1u CO-stretching manifold in ground state Cr(CO)(6) induces loss of CO. Enhancement and inhibition, respectively, of the dissociation are demonstrated by applying negative or positive chirp to the pulses.

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