Photosensitization of Single-Crystal ZnO by a Conjugated Polyelectrolyte Designed to Avoid Aggregation
JOURNAL OF PHYSICAL CHEMISTRY LETTERS(2013)
摘要
A conjugated polyelectrolyte (CPE) based on a poly(phenylene ethynylene) backbone designed to avoid interchain aggregation was adsorbed onto n-type zinc oxide (0001) single crystals. Photophysical, atomic force microscopy, and photoelectrochemical measurements confirm the absence of aggregation in solution and on ZnO single-crystal surfaces. At high surface coverage on the ZnO surface, individual polymer chains are resolved, and photocurrent efficiency measurements suggest that charge injection occurs with modest efficiency.
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关键词
conjugated polyelectrolyte,zno,single-crystal
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