Stereoselective synthesis of N-aryl proline amides by biotransformation-Ugi-Smiles sequence.

Anass Znabet,Sara Blanken,Elwin Janssen,Frans J J de Kanter,Madeleine Helliwell,Nicholas J Turner,Eelco Ruijter,Romano V A Orru

ORGANIC & BIOMOLECULAR CHEMISTRY（2012）

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摘要

An efficient combination of MAO-N-catalyzed desymmetrization of cyclic meso-amines with Ugi-Smiles multicomponent chemistry produced optically pure N-aryl proline amides. This method represents the first report of a fully asymmetric Ugi-Smiles process.

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