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π-Conjugated molecules are an important class of compounds that are used to produce organic electronics, dyes, sensors, and liquid crystal displays. Incorporation of heteroatoms into a π-conjugated skeleton is a promising way to modulate their physical properties, and thus, intensive efforts have been devoted to the construction of new hetero-π-conjugated frameworks. Because of the lack of a suitable synthetic methodology, only a few π-conjugated molecules with ring junction heteroatoms have been synthesized to date, even though numerous theoretical investigations suggested that those hetero-π-conjugated molecules could be attractive substructures of heteroatom-embedded nanocarbons. Recently, we have developed efficient carbon-heteroatom bond formation reactions, such as hetero Friedel-Crafts reaction, which can provide a facile access to π-conjugated molecules with ring junction heteroatoms. The molecules show attractive physical properties such as fluorescence and charge transport, and can be applied to the field of (opto)electronics. Molecules with such frameworks are not only attractive functional materials but also potential starting compounds for the controlled synthesis of heteroatom-embedded nanocarbons (i.e. heteronanographene) by surface-assisted coupling or amplification sheet growth.
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CHEMICAL SOCIETY REVIEWSno. 3 (2024): 1624-1692
Yi-Ting Lee,Chin-Yiu Chan, Nanami Matsuno, Shigetada Uemura,Susumu Oda, Masakazu Kondo, Rangani Wathsala Weerasinghe, Yanmei Hu, Gerardus N Iswara Lestanto,Youichi Tsuchiya, Yufang Li,Takuji Hatakeyama,
Nature communicationsno. 1 (2024): 3174-3174
Xun Tang, Mingchen Xie,Zesen Lin, Kirill Mitrofanov, Tuul Tsagaantsooj,Yi-Ting Lee,Ryota Kabe,Atula S. D. Sandanayaka,Toshinori Matsushima,Takuji Hatakeyama,Chihaya Adachi
ANGEWANDTE CHEMIE-INTERNATIONAL EDITIONno. 2 (2024): e202315210-e202315210
Junki Ochi,Yuki Yamasaki, Kojiro Tanaka,Yasuhiro Kondo, Kohei Isayama,Susumu Oda,Masakazu Kondo,Takuji Hatakeyama
Nature communicationsno. 1 (2024): 2361-2361
Yusuke Sano, Toshiki Shintani,Masahiro Hayakawa,Susumu Oda,Masakazu Kondo,Takeshi Matsushita,Takuji Hatakeyama
Journal of the American Chemical Societyno. 21 (2023): 11504-11511
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Chemistry – A European Journalno. 5 (2023)
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