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The main objectives of our research program at the University of Arizona are twofold: 1) Development and study of useful new synthetic strategies and methods for organic chemistry. 2) Total synthesis of complex natural products exhibiting unique biological activity. In our laboratory these two research areas are usually closely linked. All of our synthetic blueprints are expected to showcase a new synthetic method or a unique disconnection that is ideally suited for the target architecture thus ensuring a short and efficient synthesis, which in turn provides us with access to valuable intermediates and products for deciphering molecular mechanisms and biological evaluation. By adhering to such stringent design criteria, we find without exception that a fertile environment for new ideas is invariably created. The harmony between new reaction development and natural product total synthesis serves also to showcase the strengths of the new method over existing methods while at the same time enabling access to the natural product. It is important also not to forget that in addition to the valuable training that total synthesis provides students, the unanticipated challenges and the realization of limitations of existing methods that most good synthetic plans are faced with constantly remind us that the richest source of new ideas is often the synthetic journey itself.
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POLYMER (2024): 126539
Jianhua Bao,Kyung-Seok Kang, Jake Molineux, Derek Bischoff,Michael Mackay, Jeffrey Pyun,Jon Njardarson
ANGEWANDTE CHEMIE-INTERNATIONAL EDITIONno. 7 (2024): e202315963-e202315963
Jianhua Bao, Steven J. Nick, Aleksey S. Lanin, Nerea Iragorri Molinero, Brendon J. Sera,Jon T. Njardarson
The Journal of organic chemistryno. 24 (2023): 17485-17488
Journal of the American Chemical Societyno. 22 (2023): 12386-12397
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JOURNAL OF THE AMERICAN CHEMICAL SOCIETYno. 50 (2023): 27821-27829
Comprehensive Heterocyclic Chemistry IVpp.199-274, (2022)
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